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Smackover, Arkansas. Smackover is a small city in Union County, Arkansas, United States. According to Citydata.com, the 2014 population was at 1,790.
According to Ernie Deaneâs Arkansas Place Names, âEvidence is strong that Smackover can credit the French for its name. This is despite popular legends that tell of oil blowing âsmack over the derrick,â or a pioneer settler jumping âsmack overâ the creek, etc.