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If you were travelling in a mid range car that averaged 40 MPG and were paying Â£4.54 per gallon (1.00 per litre) for your petrol then the cost for this trip based on an estimated driving distance of 545.67 miles (830.34 kms) , from Granada to Barcelona for your fuel would be in the region of Â£61.93 .
The driving distance from Madrid to Barcelona is approximately 4-1/2 to 5 hours, unless you stop for lunch along the way, which I suggest. You follow the NII/E90 out of Madrid to Zaragoza before taking the A2/E90 to Lleida and finally into Barcelona. You'd be advised to purchase the Michelin Regional Map #572 which covers this are in detail.