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When you crack your knuckles, you're actually doing more bursting than cracking. The popping noise you hear is caused by small bubbles bursting in your synovial fluid, a yolk-like substance that lubricates the areas between bones and reduces friction for ease of movement.
Back in April, researchers from the University of Alberta published a paper based on MRI imaging of finger joints being cracked saying that the popping sound is caused by the collapse of air bubbles that form in the fluid that surrounds our joints - called synovial fluid.