Uranium
Uranium-238 is the most stable isotope of uranium, with a half-life of about 4.468 years, roughly the age of the Earth. Uranium-235 has a half-life of about 7.13 years, and uranium-234 has a half-life of about 2.48 years.
For natural uranium, about 49% of its alpha rays are emitted by each of U atom, and also 49% by U (since the latter is formed from the former) and about 2.0% of them by the U. When the Earth was young, probably about one-fifth of its uranium was uranium-235, but the percentage of U was probably much lower than this.
Isotopes of polonium
Polonium (Po) has 42 isotopes, all of which are radioactive, with between 186 and 227 nucleons. Po with a half-life of 138.376 days has the longest half-life of naturally occurring polonium. Po with a half-life of 125 years has the longest half-life of all isotopes of polonium. Po and Po (half-life 2.9 years) can be made through proton bombardment of bismuth in a cyclotron.