To further understand the magnetic behavior at low temperature, we have also performed GISANS experiments with limited intensity available, as the beamline is not optimized for this method. The signal‐to‐background ratio is not large enough to observe distinguishable features in the reciprocal space map (see Figure S2, Supporting Information). We have performed integrations along the Q y axis using a band from Q z = 0.025 Å−1−0.045 Å−1 for the models depicted in Figure 3 and the measured data, which are shown in Figure 4 . The 300 K data have a clear peak around Q y = 0.02 Å−1, which corresponds to the nuclear structure as well as the total scattering in the gas and ice‐1 states. Upon cooling down to 7 K, additional intensity develops around Q y ≈ 0.012 Å−1 that is only expected for the ice‐2 and/or the spin solid states (also see Figures S3–S5, Supporting Information for detail simulations). For the sample to manifest an Ice‐2 state, a finite intensity at Q y ≈ 0.025 Å−1 should have been observed. Rather, it is missing in the experimental data. The observed intensity profile, albeit limited, is reasonably consistent with the predicted q‐dependence of intensity in the spin solid state or, a phase mixture of spin solid state (majority phase) with ice states (minority phase).