He was a career-best third at his country event, the 2010 Ypres Rally. His final three events for the season were the 2010 Czech Rally, 2010 Rallye Sanremo and 2010 Rally Scotland. He retired in the Czech and Scottish rallies. In Sanremo he was eight, securing the final points position. Neuville finished the season in ninth place, collecting twelve points across his six events. Neuville continued with the Peugeot Bel-Lux team in the 2011 Intercontinental Rally Challenge. At the season opener in Monte Carlo he crashed his 207 S2000 in the first stage and retired. After Monte Carlo, co-driver Klinger was replaced with Nicolas Gilsoul for the rest of the season. In the next event, 2011 Rally Islas Canarias, Neuville battled for the win but finished third behind winner Juho Hänninen and second placed Jan Kopecký. First victory came in the following at event in 2011 Tour de Corse with a convincing drive, finishing 15.5 seconds in front of Kopecký. He was the early pacesetter at the following 2011 Prime Yalta Rally but going off road and a puncture meant the Belgian could only finish in sixth position. At the 2011 Ypres Rally, suspension damage resulted in retirement. At the following 2011 Czech Rally, Neuville was fourth. In Hungary, the 2011 Mecsek Rallye, Neuville was just 0.8 seconds shy of winning the rally, behind winner Kopecký. His second victory would arrive in 2011 Rallye Sanremo, winning by just 1.5 seconds. In the penultimate round in Scotland, Neuville was sixth, having spun and dropped time to the leaders. Heading into the finale in Cyprus, Neuville was one of five drivers who were able to win the title. Neuville held the rally lead early on, but soon after, an issue with the alternator on his car developed and the Belgian had to retire. The title eventually went to Andreas Mikkelsen, who won the rally, while Neuville finished fifth in the standings. Citroën signed Neuville for the 2012 World Rally Championship, driving selected races in a Citroën DS3 WRC for their junior team. The season saw Neuville make his World Rally Car-debut. At the season opener in Monte Carlo, Neuville crashed out of the event early. He remained scoreless until the fourth round in Portugal where he finished in eight position.