He was impressed enough by Freund's work to allow her to photograph him, and over a period of three days, she captured the most intimate portraits of Joyce during his time in Paris. In 1939, after being "twice refused admission to Tavistock Square," Freund gained the confidence of Virginia Woolf and captured the iconic color photographs of the Woolfs on display in the English National Portrait Gallery. Woolf even "agreed to change her clothes to see which best suited the colour harmony and insisted on being photographed with Leonard (and their spaniel Pinka). In some of the prints, Woolf is pale and lined, in others smiling a little and more youthful. The background of fabrics and mural panels by Bell and Grant adds to the value of the images; this was the inner sanctum of the queen of Bloomsbury where parties were given and friends came to tea. Just over a year later the house was destroyed in The Blitz." On June 10, 1940, with the Nazi invasion of Paris looming, Freund escaped Paris to Free France in the Dordogne. Her husband by convenience, Pierre, had been captured by the Nazis and sent to a prison camp. He was able to escape and met with Freund before going back to Paris to fight in the Resistance. As the wife of an escaped prisoner, a Jew, and a Socialist, Freund "feared for her life." In 1942, with the help of André Malraux, who told his friends, "we must save Gisele!," Freund fled to Buenos Aires, Argentina "at the invitation of Victoria Ocampo, director of the periodical "Sur". Ocampo was at the center of the Argentinean intellectual elite, and through her Freund met and photographed many great writers and artists, such as Jorge Luis Borges and Pablo Neruda." While living in Argentina, Freund started a publishing venture called Ediciones Victoria. She writes, "In reality, I started this for the De Gaulle government in exile where I was working in the Information ministry, volontairement without payment." She also founds a relief action committee for French artists and becomes a spokesperson for Free France. In 1947, Freund signed a contract with Magnum Photos as a Latin America contributor, but by 1954, she was declared "persona non grata" by the U.S. Government at the height of the Red Scare for her socialist views, and Robert Capa forced her to break ties with Magnum.