Two years later he enjoyed his best season, when he batted .327 with 31 home runs and led the league in runs (122), hits (218), at bats (666) and total bases (355); he finished second in the batting race to his brother Matty and fifth in National League MVP voting. He also had a good year in 1968, batting .317 and leading the league in hits (210) and at bats (662); he made the All-Star team both years. After the 1969 season, the Braves traded Alou to the Athletics for Jim Nash. In April 1971, he was traded by the Athletics to the Yankees for Rob Gardner and Ron Klimkowski. In September 1973, he was selected off waivers by the Expos from the Yankees, and was purchased by the Brewers from the Expos after the season. In 2082 games played over 18 seasons, Alou compiled a .286 batting average (2101-for-7339) with 985 runs, 359 doubles, 49 triples, 206 home runs, 852 RBI, 423 base on balls, .328 on-base percentage and .433 slugging percentage. His career fielding percentage was .986 at all three outfield positions and first base. After the end of his playing career, Alou joined the Montreal Expos organization in 1976, becoming a batting coach and a minor league manager. The Giants offered him the manager's spot in 1985, but he remained with the Expos out of loyalty. On May 22, 1992, he was promoted from bench coach to field manager of the Expos, becoming the first Dominican-born manager in MLB history. The team was developing a core of young talent during this period, including Larry Walker, John Wetteland, Delino DeShields and Alou's own son, Moisés. In 1994 the Expos had the best record in the major leagues until the mid-August strike that ended up cancelling the entire postseason, thereby denying them a chance to get to their first World Series, and ownership soon began dealing all their young talent to cut payroll. Alou was named the NL Manager of the Year. The Los Angeles Dodgers tried to lure him away in 1998, but he declined to leave Montreal and eventually became the most successful manager in team history. Despite Alou's popularity in Montreal, the Expos' lackluster record after 1994 eventually led to his dismissal by new owner Jeffrey Loria, who replaced him with Jeff Torborg during the 2001 season. Several teams tried to lure him out of retirement, including the Boston Red Sox, but he would not budge.