Is anything inherently random? Is anything inherently random? Or is all randomness observed in data either "errors in measurement" or "lack of understanding"? Assume we could measure everything with infinite precision and had a complete understanding of all the deterministic processes. Would there be any process that would appear "random" in the data or would every dataset be deterministic at that point?

Independently of the question of existence of randomness, you simply cannot measure anything to arbitrarily high precision, because your measurement will necessarily disturb it by a greater amount if you wish to have greater precision. This is already true in classical mechanics and remains true in quantum mechanics.
But your real question is whether there is anything inherently random in the world. Although this is not a mathematical question, it suffices to say that till today there is simply zero evidence for any truly random process. Quantum mechanics does not at all suggest, not to say imply, randomness in anything in the real world. Given this, it is reasonable to ask why so many real-world processes do appear to be probabilistic.
Well, the answer is that purely deterministic processes can amplify very small perturbations, so if there is an amplification process followed by a folding process then the result can appear chaotic even if it is fully determined by the initial state. Furthermore, symmetries in the folding process may strongly dictate the limiting distribution of the result as the amplification is increased.
For example, the logistic map has chaotic behaviour for certain parameters, for which just a slight perturbation in the input results in exponential divergence of the output. Essentially, the logistic map shows that repeated application of a continuous stretch-and-fold operation on a metric space can result in unpredictability in the limit. This has implications for the real-world, in that almost all measurements are of quantities arising from innumerable iterates of some physical process (e.g. particle-particle interactions).
