Calculate the transition dipole moments between the 1s inner shell and the high-lying states of a molecule

I am trying to calculate the transition dipole moments between the 1s inner shell and the high-lying states of N2, namely, $<\psi\_{1s}|{\bf r}|\psi\_{high-lying}>$. 


For this, I installed GAMESS (US) and calculated molecular orbitals of N2.  

However, I only got HOMO-6 to LUMO+2.  

I want LUMO+3, 4, 5... and if possible, 1s.


How can I do this in GAMESS? Or do I need other softwares?




Might have found the option you are looking for. GAMESS controls MO printing with the `NPREO` keyword. If you can specify ranges of orbitals either by their number (e.g. `NPREO(1)=1,10` prints the first 10 orbitals) or relative to the HOMO (e.g. `NPREO(1)=-3,-5` prints from HOMO-3 to LUMO+4). You can also give 3rd and 4th numbers to list the range of orbital energies to print.


These print options are described on p.23 of the [input descriptions](https://www.msg.chem.iastate.edu/gamess/documentation.html) document on the Gordon research group page.


 1