  We report a novel crossover behavior in the long-range-ordered phase of a
prototypical spin-$1/2$ Heisenberg antiferromagnetic ladder compound
$\mathrm{(C_7H_{10}N)_2CuBr_4}$. The staggered order was previously evidenced
from a continuous and symmetric splitting of $^{14}$N NMR spectral lines on
lowering temperature below $T_c\simeq 330$ mK, with a saturation towards
$\simeq 150$ mK. Unexpectedly, the split lines begin to further separate away
below $T^*\sim 100$ mK while the line width and shape remain completely
invariable. This crossover behavior is further corroborated by the NMR
relaxation rate $T_1^{-1}$ measurements. A very strong suppression reflecting
the ordering, $T_1^{-1}\sim T^{5.5}$, observed above $T^*$, is replaced by
$T_1^{-1}\sim T$ below $T^*$. These original NMR features are indicative of
unconventional nature of the crossover, which may arise from a unique
arrangement of the ladders into a spatially anisotropic and frustrated coupling
network.

Strongly Correlated Electrons