Empirical models for particulate matter emissions from paved road surfaces have been criticised for their lack of realism and accuracy. To support the development of a less empirical model, a study was conducted in a busy street at the DAPPLE site in Central London to understand the processes and to identify important parameters that influence emission from paved roads. Ordinary road gritting salt was applied to the road and the particulate matter entering the air at near-road surface level was monitored using optical particle counters. The grit acted as a tracer. The grit moved rapidly along the road in the direction of traffic flow. Build-up of material at the kerb indicated material being thrown across the road by the traffic. Coarser particles were resuspended faster than the finer ones. A clear decay profile was seen in the case of particles larger than 2 μ m ; particles smaller than 2 μ m did not show any decay pattern during the experiment duration. Grinding of material appears to control the reservoir of fine particles on the road surface. The amount of material resuspended by traffic is about 30% less than those removed along the road and a factor of 6 higher than the amount removed across the road. Resuspension accounts for 40% of the total material removed from a road segment and 70% of the material removed together along and across the road. On average a single vehicle pass removes 0.08% of material present on a road segment at that instant. The calculation scheme is obtained from a short-duration study and therefore further studies of long duration involving varying road geometry and different traffic and meteorological condition need to be carried out before applying parameter estimates presented in this paper.