This paper details the enhancements in the dielectric and piezoelectric properties of a low-temperature screen-printable piezoelectric nano-composite film on flexible plastic and textile substrates. These enhancements involved adding silver nano particles to the nano-composite material and using an additional cold isostatic pressing (CIP) post-processing procedure. These developments have resulted in a 18% increase in the free-standing piezoelectric charge coefficient d33 to a value of 98 pC/N. The increase in the dielectric constant of the piezoelectric film has, however, resulted in a decrease in the peak output voltage of the composite film. The potential for this material to be used to harvest mechanical energy from a variety of textiles under compressive and bending forces has been evaluated theoretically and experimentally. The maximum energy density of the enhanced piezoelectric material under 800N compressive force was found to be 34J/m3 on a Kermel textile. The maximum energy density of the enhanced piezoelectric material under bending was found to be 14.3J/m3 on a cotton textile. These results agree very favourably with the theoretical predictions. For a 10x10cm piezoelectric element 100µm thick this equates to 38μJ and 14.3μJ of energy generated per mechanical action respectively which is a potentially useful amount of energy.